By Kasper Moth-Poulsen
Single-molecule electronics has advanced as a colourful study box over the past twenty years. The imaginative and prescient is for you to create digital elements on the maximum point of miniaturization―the unmarried molecule. This e-book compiles and information state of the art examine with contributions from chemists, physicists, theoreticians, and engineers. It covers all elements of single-molecule electronics, from the speculation via experimental realizations and the chemical synthesis of molecular parts to the implementation of molecular elements in destiny built-in circuits.
This booklet describes intimately either verified equipment and up to date advances within the box, together with vibrational results, switching phenomena, quantum interference, thermal energy, and parallel meeting suggestions. The authors upload extra info to the chapters than in general present in the first literature in order that the publication should be learn not just by means of experts but in addition by way of non-experts and scholars with an curiosity within the examine box. each one bankruptcy is followed through difficulties, and a recommendations guide is additionally provided.
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Single-molecule electronics has advanced as a colourful learn box over the past 20 years. The imaginative and prescient is in order to create digital elements on the maximum point of miniaturization―the unmarried molecule. This publication compiles and info state-of-the-art learn with contributions from chemists, physicists, theoreticians, and engineers.
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Additional resources for Handbook of Single-molecule Electronics
Physical Review B, 1999. 59(19): pp. 12505–12513. 37. , Lithographic mechanical break junctions for singlemolecule measurements in vacuum: possibilities and limitations. New Journal of Physics, 2008. 10: p. 065008. 38. Moreland, J. W. Ekin, Electron-tunneling experiments using NbSn break junctions. Journal of Applied Physics, 1985. 58(10): pp. 3888– 3895. 39. , Conductance of a molecular junction. Science, 1997. 278(5336): pp. 252–254. 40. , Adjustable nanofabricated atomic size contacts. Review of Scientiﬁc Instruments, 1996.
67(1): pp. 108–111. 41. , A versatile low-temperature setup for the electrical characterization of single-molecule junctions. Review of Scientiﬁc Instruments, 2011. 82(5): p. 8. © 2016 by Taylor & Francis Group, LLC July 1, 2015 12:58 PSP Book - 9in x 6in 02-Kasper-Moth-Poulsen-c02 28 Experimental Techniques 42. , An electrochemically assisted mechanically controllable break junction approach for single molecule junction conductance measurements. Nano Research, 2011. 4(12): pp. 1199–1207. 43. , Molecular junctions based on intermolecular electrostatic coupling.
In the example above, where N = 6, and for other small systems (a couple of hundred atoms), this would pose no problem, but if we were to increase the system size even further, we would soon run into trouble since the time required for the matrix inversion would grow too large. Thus, we require a more eﬃcient way of calculating the Green’s functions than the “brute force” method based on direct inversion of the full system’s Hamiltonian. This is where the recursive Green’s function method comes into play.